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Moving artificial leaves out of the lab and into the air
https://today.uic.edu/moving-artificial-leaves-out-of-the-lab-and-into-the-airMoving artificial leaves out of the lab and into the air
February 12, 2019
Artificial leaves mimic photosynthesis — the process whereby plants use water and carbon dioxide from the air to produce carbohydrates using energy from the sun. But even state-of-the-art artificial leaves, which hold promise in reducing carbon dioxide from the atmosphere, only work in the laboratory because they use pure, pressurized carbon dioxide from tanks.
But now, researchers from the University of Illinois at Chicago have proposed a design solution that could bring artificial leaves out of the lab and into the environment. Their improved leaf, which would use carbon dioxide — a potent greenhouse gas — from the air, would be at least 10 times more efficient than natural leaves at converting carbon dioxide to fuel. Their findings are reported in the journal ACS Sustainable Chemistry & Engineering.
“So far, all designs for artificial leaves that have been tested in the lab use carbon dioxide from pressurized tanks. In order to implement successfully in the real world, these devices need to be able to draw carbon dioxide from much more dilute sources, such as air and flue gas, which is the gas given off by coal-burning power plants,” said Meenesh Singh, assistant professor of chemical engineering in the UIC College of Engineering and corresponding author on the paper.
…
Singh and his colleague Aditya Prajapati, a graduate student in his lab, proposed solving this problem by encapsulating a traditional artificial leaf inside a transparent capsule made of a semi-permeable membrane of quaternary ammonium resin and filled with water. The membrane allows water from inside to evaporate out when warmed by sunlight. As water passes out through the membrane, it selectively pulls in carbon dioxide from the air. The artificial photosynthetic unit inside the capsule is made up of a light absorber coated with catalysts that convert the carbon dioxide to carbon monoxide, which can be siphoned off and used as a basis for the creation of various synthetic fuels. Oxygen is also produced and can either be collected or released into the surrounding environment.
…
https://dx.doi.org/10.1021/acssuschemeng.8b04969February 12, 2019
Artificial leaves mimic photosynthesis — the process whereby plants use water and carbon dioxide from the air to produce carbohydrates using energy from the sun. But even state-of-the-art artificial leaves, which hold promise in reducing carbon dioxide from the atmosphere, only work in the laboratory because they use pure, pressurized carbon dioxide from tanks.
But now, researchers from the University of Illinois at Chicago have proposed a design solution that could bring artificial leaves out of the lab and into the environment. Their improved leaf, which would use carbon dioxide — a potent greenhouse gas — from the air, would be at least 10 times more efficient than natural leaves at converting carbon dioxide to fuel. Their findings are reported in the journal ACS Sustainable Chemistry & Engineering.
“So far, all designs for artificial leaves that have been tested in the lab use carbon dioxide from pressurized tanks. In order to implement successfully in the real world, these devices need to be able to draw carbon dioxide from much more dilute sources, such as air and flue gas, which is the gas given off by coal-burning power plants,” said Meenesh Singh, assistant professor of chemical engineering in the UIC College of Engineering and corresponding author on the paper.
…
Singh and his colleague Aditya Prajapati, a graduate student in his lab, proposed solving this problem by encapsulating a traditional artificial leaf inside a transparent capsule made of a semi-permeable membrane of quaternary ammonium resin and filled with water. The membrane allows water from inside to evaporate out when warmed by sunlight. As water passes out through the membrane, it selectively pulls in carbon dioxide from the air. The artificial photosynthetic unit inside the capsule is made up of a light absorber coated with catalysts that convert the carbon dioxide to carbon monoxide, which can be siphoned off and used as a basis for the creation of various synthetic fuels. Oxygen is also produced and can either be collected or released into the surrounding environment.
…
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